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Supramolecular assembly on surfaces: manipulating conductance in noncovalently modified mesoscale structures. 2002
Grace M Credo, and
Andrew K Boal, and
Kanad Das, and
Trent H Galow, and
Vincent M Rotello, and
Daniel L Feldheim, and
Christopher B Gorman
Department of Chemistry, North Carolina State University, Raleigh, North Carolina 27695, USA.
Molecules capable of complementary hydrogen bonding were used to control the noncovalent self-assembly and electronic properties of a chemically well-defined surface mesostructure. In this work, we patterned a footprint region for molecular assembly on a surface and used moieties featuring complementary recognition to tune the current-voltage properties of the patterned region. With the appropriate functionalities on the complementary moieties, we were able to increase and decrease the observed conductance in surface-bound mesoscale structures imaged by scanning tunneling microscopy (STM).
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