Determination of Henry's law constants for low volatile mixed halogenated anisoles using solid-phase microextraction. 2007

Alfredo Diaz, and Francesc Ventura, and Maria Teresa Galceran
AGBAR, Societat General d'Aigües de Barcelona, Barcelona, Spain. adiazbanos@agbar.es <adiazbanos@agbar.es>

Trihalogenated anisoles (THAs) that have been identified at low concentration levels (ngL(-1)) in drinking water are suspected of causing odor episodes, which are a frequent source of complaint by consumers. Henry's law constant (K(H)) is an important parameter in controlling the diffusion of organic compounds from the water to the vapor-phase, so its evaluation is of significance in the study of odor events. In this paper, the K(H) of a wide range of trihalogenated anisoles--in its dimensionless form [Formula: see text]--were calculated at two temperatures, 45 and 22 degrees C using equilibration partitioning in a closed system and headspace microextraction (EPICS-SPME). Two methodological approaches, Ramachandran and Dewulf, were used for the assessment of the Henry's law constant. Nevertheless, to apply these methods to THAs, a relatively narrow headspace/water volume ratio range (80/1-8/1) is required. At these conditions, a linearity (r(2)) using Ramachandran's theoretical relationship from 0.9276 to 0.9989 was obtained and the variability (R.S.D.%) when Dewulf's theoretical relationship was employed was lower than 20% (n=5).

UI MeSH Term Description Entries
D012015 Reference Standards A basis of value established for the measure of quantity, weight, extent or quality, e.g. weight standards, standard solutions, methods, techniques, and procedures used in diagnosis and therapy. Standard Preparations,Standards, Reference,Preparations, Standard,Standardization,Standards,Preparation, Standard,Reference Standard,Standard Preparation,Standard, Reference
D000840 Anisoles A group of compounds that are derivatives of methoxybenzene and contain the general formula R-C7H7O. Methylphenyl Ethers,Ethers, Methylphenyl
D014835 Volatilization A phase transition from liquid state to gas state, which is affected by Raoult's law. It can be accomplished by fractional distillation. Vaporization,Volatility
D014881 Water Supply Means or process of supplying water (as for a community) usually including reservoirs, tunnels, and pipelines and often the watershed from which the water is ultimately drawn. (Webster, 3d ed) Supplies, Water,Supply, Water,Water Supplies

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