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Multiphoton electron angular distributions from laser-aligned CS2 molecules. 2008
Vinod Kumarappan, and
Lotte Holmegaard, and
Christian Martiny, and
Christian B Madsen, and
Thomas K Kjeldsen, and
Simon S Viftrup, and
Lars Bojer Madsen, and
Henrik Stapelfeldt
Department of Chemistry, University of Aarhus, 8000 Aarhus C, Denmark.
Laser-aligned carbondisulfide (CS2) molecules are singly ionized by multiphoton absorption from intense, linearly polarized 25 fs laser pulses. The angular distribution of the photoelectrons exhibits a significant dependence on the angle between the polarizations of the aligning and ionizing laser fields. The widely used strong-field approximation predicts angular distributions in qualitative agreement with the experimental data but fails at a quantitative level.
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