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Factors influencing the optical bandwidth of a free-running pulsed beta-barium borate optical parametric oscillator are examined and incorporated in a simple fitting procedure. Spatiospectral phenomena in the optical parametric oscillator output beam are thereby identified; these suggest a novel way to reduce the effective optical bandwidth for spectroscopic purposes. This technique is demonstrated by recording a degenerate fourwave mixing spectrum of sodium atoms in an air-acetylene flame.
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