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Evolution of organic aerosols in the atmosphere. 2009
J L Jimenez, and
M R Canagaratna, and
N M Donahue, and
A S H Prevot, and
Q Zhang, and
J H Kroll, and
P F DeCarlo, and
J D Allan, and
H Coe, and
N L Ng, and
A C Aiken, and
K S Docherty, and
I M Ulbrich, and
A P Grieshop, and
A L Robinson, and
J Duplissy, and
J D Smith, and
K R Wilson, and
V A Lanz, and
C Hueglin, and
Y L Sun, and
J Tian, and
A Laaksonen, and
T Raatikainen, and
J Rautiainen, and
P Vaattovaara, and
M Ehn, and
M Kulmala, and
J M Tomlinson, and
D R Collins, and
M J Cubison, and
E J Dunlea, and
J A Huffman, and
T B Onasch, and
M R Alfarra, and
P I Williams, and
K Bower, and
Y Kondo, and
J Schneider, and
F Drewnick, and
S Borrmann, and
S Weimer, and
K Demerjian, and
D Salcedo, and
L Cottrell, and
R Griffin, and
A Takami, and
T Miyoshi, and
S Hatakeyama, and
A Shimono, and
J Y Sun, and
Y M Zhang, and
K Dzepina, and
J R Kimmel, and
D Sueper, and
J T Jayne, and
S C Herndon, and
A M Trimborn, and
L R Williams, and
E C Wood, and
A M Middlebrook, and
C E Kolb, and
U Baltensperger, and
D R Worsnop
Cooperative Institute for Research in the Environmental Sciences and Department of Chemistry and Biochemistry, University of Colorado, Boulder, CO, USA. jose.jimenez@colorado.edu
Organic aerosol (OA) particles affect climate forcing and human health, but their sources and evolution remain poorly characterized. We present a unifying model framework describing the atmospheric evolution of OA that is constrained by high-time-resolution measurements of its composition, volatility, and oxidation state. OA and OA precursor gases evolve by becoming increasingly oxidized, less volatile, and more hygroscopic, leading to the formation of oxygenated organic aerosol (OOA), with concentrations comparable to those of sulfate aerosol throughout the Northern Hemisphere. Our model framework captures the dynamic aging behavior observed in both the atmosphere and laboratory: It can serve as a basis for improving parameterizations in regional and global models.
| UI | MeSH Term | Description | Entries |
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Related Publications
J L Jimenez, and
M R Canagaratna, and
N M Donahue, and
A S H Prevot, and
Q Zhang, and
J H Kroll, and
P F DeCarlo, and
J D Allan, and
H Coe, and
N L Ng, and
A C Aiken, and
K S Docherty, and
I M Ulbrich, and
A P Grieshop, and
A L Robinson, and
J Duplissy, and
J D Smith, and
K R Wilson, and
V A Lanz, and
C Hueglin, and
Y L Sun, and
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T Raatikainen, and
J Rautiainen, and
P Vaattovaara, and
M Ehn, and
M Kulmala, and
J M Tomlinson, and
D R Collins, and
M J Cubison, and
E J Dunlea, and
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M R Alfarra, and
P I Williams, and
K Bower, and
Y Kondo, and
J Schneider, and
F Drewnick, and
S Borrmann, and
S Weimer, and
K Demerjian, and
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R Griffin, and
A Takami, and
T Miyoshi, and
S Hatakeyama, and
A Shimono, and
J Y Sun, and
Y M Zhang, and
K Dzepina, and
J R Kimmel, and
D Sueper, and
J T Jayne, and
S C Herndon, and
A M Trimborn, and
L R Williams, and
E C Wood, and
A M Middlebrook, and
C E Kolb, and
U Baltensperger, and
D R Worsnop
October 2009,
Environmental science & technology,
J L Jimenez, and
M R Canagaratna, and
N M Donahue, and
A S H Prevot, and
Q Zhang, and
J H Kroll, and
P F DeCarlo, and
J D Allan, and
H Coe, and
N L Ng, and
A C Aiken, and
K S Docherty, and
I M Ulbrich, and
A P Grieshop, and
A L Robinson, and
J Duplissy, and
J D Smith, and
K R Wilson, and
V A Lanz, and
C Hueglin, and
Y L Sun, and
J Tian, and
A Laaksonen, and
T Raatikainen, and
J Rautiainen, and
P Vaattovaara, and
M Ehn, and
M Kulmala, and
J M Tomlinson, and
D R Collins, and
M J Cubison, and
E J Dunlea, and
J A Huffman, and
T B Onasch, and
M R Alfarra, and
P I Williams, and
K Bower, and
Y Kondo, and
J Schneider, and
F Drewnick, and
S Borrmann, and
S Weimer, and
K Demerjian, and
D Salcedo, and
L Cottrell, and
R Griffin, and
A Takami, and
T Miyoshi, and
S Hatakeyama, and
A Shimono, and
J Y Sun, and
Y M Zhang, and
K Dzepina, and
J R Kimmel, and
D Sueper, and
J T Jayne, and
S C Herndon, and
A M Trimborn, and
L R Williams, and
E C Wood, and
A M Middlebrook, and
C E Kolb, and
U Baltensperger, and
D R Worsnop
July 2010,
Proceedings of the National Academy of Sciences of the United States of America,
J L Jimenez, and
M R Canagaratna, and
N M Donahue, and
A S H Prevot, and
Q Zhang, and
J H Kroll, and
P F DeCarlo, and
J D Allan, and
H Coe, and
N L Ng, and
A C Aiken, and
K S Docherty, and
I M Ulbrich, and
A P Grieshop, and
A L Robinson, and
J Duplissy, and
J D Smith, and
K R Wilson, and
V A Lanz, and
C Hueglin, and
Y L Sun, and
J Tian, and
A Laaksonen, and
T Raatikainen, and
J Rautiainen, and
P Vaattovaara, and
M Ehn, and
M Kulmala, and
J M Tomlinson, and
D R Collins, and
M J Cubison, and
E J Dunlea, and
J A Huffman, and
T B Onasch, and
M R Alfarra, and
P I Williams, and
K Bower, and
Y Kondo, and
J Schneider, and
F Drewnick, and
S Borrmann, and
S Weimer, and
K Demerjian, and
D Salcedo, and
L Cottrell, and
R Griffin, and
A Takami, and
T Miyoshi, and
S Hatakeyama, and
A Shimono, and
J Y Sun, and
Y M Zhang, and
K Dzepina, and
J R Kimmel, and
D Sueper, and
J T Jayne, and
S C Herndon, and
A M Trimborn, and
L R Williams, and
E C Wood, and
A M Middlebrook, and
C E Kolb, and
U Baltensperger, and
D R Worsnop
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Environmental science & technology,
J L Jimenez, and
M R Canagaratna, and
N M Donahue, and
A S H Prevot, and
Q Zhang, and
J H Kroll, and
P F DeCarlo, and
J D Allan, and
H Coe, and
N L Ng, and
A C Aiken, and
K S Docherty, and
I M Ulbrich, and
A P Grieshop, and
A L Robinson, and
J Duplissy, and
J D Smith, and
K R Wilson, and
V A Lanz, and
C Hueglin, and
Y L Sun, and
J Tian, and
A Laaksonen, and
T Raatikainen, and
J Rautiainen, and
P Vaattovaara, and
M Ehn, and
M Kulmala, and
J M Tomlinson, and
D R Collins, and
M J Cubison, and
E J Dunlea, and
J A Huffman, and
T B Onasch, and
M R Alfarra, and
P I Williams, and
K Bower, and
Y Kondo, and
J Schneider, and
F Drewnick, and
S Borrmann, and
S Weimer, and
K Demerjian, and
D Salcedo, and
L Cottrell, and
R Griffin, and
A Takami, and
T Miyoshi, and
S Hatakeyama, and
A Shimono, and
J Y Sun, and
Y M Zhang, and
K Dzepina, and
J R Kimmel, and
D Sueper, and
J T Jayne, and
S C Herndon, and
A M Trimborn, and
L R Williams, and
E C Wood, and
A M Middlebrook, and
C E Kolb, and
U Baltensperger, and
D R Worsnop
April 2015,
Scientific reports,
J L Jimenez, and
M R Canagaratna, and
N M Donahue, and
A S H Prevot, and
Q Zhang, and
J H Kroll, and
P F DeCarlo, and
J D Allan, and
H Coe, and
N L Ng, and
A C Aiken, and
K S Docherty, and
I M Ulbrich, and
A P Grieshop, and
A L Robinson, and
J Duplissy, and
J D Smith, and
K R Wilson, and
V A Lanz, and
C Hueglin, and
Y L Sun, and
J Tian, and
A Laaksonen, and
T Raatikainen, and
J Rautiainen, and
P Vaattovaara, and
M Ehn, and
M Kulmala, and
J M Tomlinson, and
D R Collins, and
M J Cubison, and
E J Dunlea, and
J A Huffman, and
T B Onasch, and
M R Alfarra, and
P I Williams, and
K Bower, and
Y Kondo, and
J Schneider, and
F Drewnick, and
S Borrmann, and
S Weimer, and
K Demerjian, and
D Salcedo, and
L Cottrell, and
R Griffin, and
A Takami, and
T Miyoshi, and
S Hatakeyama, and
A Shimono, and
J Y Sun, and
Y M Zhang, and
K Dzepina, and
J R Kimmel, and
D Sueper, and
J T Jayne, and
S C Herndon, and
A M Trimborn, and
L R Williams, and
E C Wood, and
A M Middlebrook, and
C E Kolb, and
U Baltensperger, and
D R Worsnop
January 1995,
Planetary and space science,
J L Jimenez, and
M R Canagaratna, and
N M Donahue, and
A S H Prevot, and
Q Zhang, and
J H Kroll, and
P F DeCarlo, and
J D Allan, and
H Coe, and
N L Ng, and
A C Aiken, and
K S Docherty, and
I M Ulbrich, and
A P Grieshop, and
A L Robinson, and
J Duplissy, and
J D Smith, and
K R Wilson, and
V A Lanz, and
C Hueglin, and
Y L Sun, and
J Tian, and
A Laaksonen, and
T Raatikainen, and
J Rautiainen, and
P Vaattovaara, and
M Ehn, and
M Kulmala, and
J M Tomlinson, and
D R Collins, and
M J Cubison, and
E J Dunlea, and
J A Huffman, and
T B Onasch, and
M R Alfarra, and
P I Williams, and
K Bower, and
Y Kondo, and
J Schneider, and
F Drewnick, and
S Borrmann, and
S Weimer, and
K Demerjian, and
D Salcedo, and
L Cottrell, and
R Griffin, and
A Takami, and
T Miyoshi, and
S Hatakeyama, and
A Shimono, and
J Y Sun, and
Y M Zhang, and
K Dzepina, and
J R Kimmel, and
D Sueper, and
J T Jayne, and
S C Herndon, and
A M Trimborn, and
L R Williams, and
E C Wood, and
A M Middlebrook, and
C E Kolb, and
U Baltensperger, and
D R Worsnop
January 1997,
Advances in space research : the official journal of the Committee on Space Research (COSPAR),
J L Jimenez, and
M R Canagaratna, and
N M Donahue, and
A S H Prevot, and
Q Zhang, and
J H Kroll, and
P F DeCarlo, and
J D Allan, and
H Coe, and
N L Ng, and
A C Aiken, and
K S Docherty, and
I M Ulbrich, and
A P Grieshop, and
A L Robinson, and
J Duplissy, and
J D Smith, and
K R Wilson, and
V A Lanz, and
C Hueglin, and
Y L Sun, and
J Tian, and
A Laaksonen, and
T Raatikainen, and
J Rautiainen, and
P Vaattovaara, and
M Ehn, and
M Kulmala, and
J M Tomlinson, and
D R Collins, and
M J Cubison, and
E J Dunlea, and
J A Huffman, and
T B Onasch, and
M R Alfarra, and
P I Williams, and
K Bower, and
Y Kondo, and
J Schneider, and
F Drewnick, and
S Borrmann, and
S Weimer, and
K Demerjian, and
D Salcedo, and
L Cottrell, and
R Griffin, and
A Takami, and
T Miyoshi, and
S Hatakeyama, and
A Shimono, and
J Y Sun, and
Y M Zhang, and
K Dzepina, and
J R Kimmel, and
D Sueper, and
J T Jayne, and
S C Herndon, and
A M Trimborn, and
L R Williams, and
E C Wood, and
A M Middlebrook, and
C E Kolb, and
U Baltensperger, and
D R Worsnop
February 2005,
Angewandte Chemie (International ed. in English),
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M R Canagaratna, and
N M Donahue, and
A S H Prevot, and
Q Zhang, and
J H Kroll, and
P F DeCarlo, and
J D Allan, and
H Coe, and
N L Ng, and
A C Aiken, and
K S Docherty, and
I M Ulbrich, and
A P Grieshop, and
A L Robinson, and
J Duplissy, and
J D Smith, and
K R Wilson, and
V A Lanz, and
C Hueglin, and
Y L Sun, and
J Tian, and
A Laaksonen, and
T Raatikainen, and
J Rautiainen, and
P Vaattovaara, and
M Ehn, and
M Kulmala, and
J M Tomlinson, and
D R Collins, and
M J Cubison, and
E J Dunlea, and
J A Huffman, and
T B Onasch, and
M R Alfarra, and
P I Williams, and
K Bower, and
Y Kondo, and
J Schneider, and
F Drewnick, and
S Borrmann, and
S Weimer, and
K Demerjian, and
D Salcedo, and
L Cottrell, and
R Griffin, and
A Takami, and
T Miyoshi, and
S Hatakeyama, and
A Shimono, and
J Y Sun, and
Y M Zhang, and
K Dzepina, and
J R Kimmel, and
D Sueper, and
J T Jayne, and
S C Herndon, and
A M Trimborn, and
L R Williams, and
E C Wood, and
A M Middlebrook, and
C E Kolb, and
U Baltensperger, and
D R Worsnop
November 2016,
The Science of the total environment,
J L Jimenez, and
M R Canagaratna, and
N M Donahue, and
A S H Prevot, and
Q Zhang, and
J H Kroll, and
P F DeCarlo, and
J D Allan, and
H Coe, and
N L Ng, and
A C Aiken, and
K S Docherty, and
I M Ulbrich, and
A P Grieshop, and
A L Robinson, and
J Duplissy, and
J D Smith, and
K R Wilson, and
V A Lanz, and
C Hueglin, and
Y L Sun, and
J Tian, and
A Laaksonen, and
T Raatikainen, and
J Rautiainen, and
P Vaattovaara, and
M Ehn, and
M Kulmala, and
J M Tomlinson, and
D R Collins, and
M J Cubison, and
E J Dunlea, and
J A Huffman, and
T B Onasch, and
M R Alfarra, and
P I Williams, and
K Bower, and
Y Kondo, and
J Schneider, and
F Drewnick, and
S Borrmann, and
S Weimer, and
K Demerjian, and
D Salcedo, and
L Cottrell, and
R Griffin, and
A Takami, and
T Miyoshi, and
S Hatakeyama, and
A Shimono, and
J Y Sun, and
Y M Zhang, and
K Dzepina, and
J R Kimmel, and
D Sueper, and
J T Jayne, and
S C Herndon, and
A M Trimborn, and
L R Williams, and
E C Wood, and
A M Middlebrook, and
C E Kolb, and
U Baltensperger, and
D R Worsnop
January 2006,
Rapid communications in mass spectrometry : RCM,
J L Jimenez, and
M R Canagaratna, and
N M Donahue, and
A S H Prevot, and
Q Zhang, and
J H Kroll, and
P F DeCarlo, and
J D Allan, and
H Coe, and
N L Ng, and
A C Aiken, and
K S Docherty, and
I M Ulbrich, and
A P Grieshop, and
A L Robinson, and
J Duplissy, and
J D Smith, and
K R Wilson, and
V A Lanz, and
C Hueglin, and
Y L Sun, and
J Tian, and
A Laaksonen, and
T Raatikainen, and
J Rautiainen, and
P Vaattovaara, and
M Ehn, and
M Kulmala, and
J M Tomlinson, and
D R Collins, and
M J Cubison, and
E J Dunlea, and
J A Huffman, and
T B Onasch, and
M R Alfarra, and
P I Williams, and
K Bower, and
Y Kondo, and
J Schneider, and
F Drewnick, and
S Borrmann, and
S Weimer, and
K Demerjian, and
D Salcedo, and
L Cottrell, and
R Griffin, and
A Takami, and
T Miyoshi, and
S Hatakeyama, and
A Shimono, and
J Y Sun, and
Y M Zhang, and
K Dzepina, and
J R Kimmel, and
D Sueper, and
J T Jayne, and
S C Herndon, and
A M Trimborn, and
L R Williams, and
E C Wood, and
A M Middlebrook, and
C E Kolb, and
U Baltensperger, and
D R Worsnop
January 2017,
Current climate change reports,
