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One pot 'click' reactions: tandem enantioselective biocatalytic epoxide ring opening and [3+2] azide alkyne cycloaddition. 2010
Lachlan S Campbell-Verduyn, and
Wiktor Szymański, and
Christiaan P Postema, and
Rudi A Dierckx, and
Philip H Elsinga, and
Dick B Janssen, and
Ben L Feringa
Stratingh Institute for Chemistry, University of Groningen, Groningen, the Netherlands.
Halohydrin dehalogenase (HheC) can perform enantioselective azidolysis of aromatic epoxides to 1,2-azido alcohols which are subsequently ligated to alkynes producing chiral hydroxy triazoles in a one-pot procedure with excellent enantiomeric excess.
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