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Two-photon absorption circular dichroism: a new twist in nonlinear spectroscopy. 2010
Carlos Toro, and
Leonardo De Boni, and
Na Lin, and
Fabrizio Santoro, and
Antonio Rizzo, and
Florencio E Hernandez
Department of Chemistry, University of Central Florida, P. O. Box 162366, Orlando, FL 32816-2366, USA.
Herein we report on the full experimental measurement of the two-photon absorption circular dichroism spectra of (S)-(-)-1,1'-bi(2-naphthol) and (R)-(+)-1,1'-bi(2-naphthol), their analysis, and theoretical support. The finding of new nonlinear optical fingerprints in chiral molecules offers new opportunities in the recognition and understanding of optically active systems in regions where CD could present strong limitations.
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