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Kinetics and dynamics of the S(1D2) + H2 → SH + H reaction at very low temperatures and collision energies. 2010
Coralie Berteloite, and
Manuel Lara, and
Astrid Bergeat, and
Sébastien D Le Picard, and
Fabrice Dayou, and
Kevin M Hickson, and
André Canosa, and
Christian Naulin, and
Jean-Michel Launay, and
Ian R Sims, and
Michel Costes
Institut de Physique de Rennes, UMR 6251 du CNRS-Université de Rennes 1, Campus de Beaulieu, 35042 Rennes Cedex, France.
We report combined studies on the prototypical S(1D2) + H2 insertion reaction. Kinetics and crossed-beam experiments are performed in experimental conditions approaching the cold energy regime, yielding absolute rate coefficients down to 5.8 K and relative integral cross sections to collision energies as low as 0.68 meV. They are supported by quantum calculations on a potential energy surface treating long-range interactions accurately. All results are consistent and the excitation function behavior is explained in terms of the cumulative contribution of various partial waves.
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