Iodine-129, iodine-127 and caesium-137 in the environment: soils from Germany and Chile. 2012

A Daraoui, and R Michel, and M Gorny, and D Jakob, and R Sachse, and H-A Synal, and V Alfimov
Institut für Radioökologie und Strahlenschutz, Leibniz Universität Hannover, Herrenhaeuser Str. 2, D-30419 Hannover, Germany. daraoui@irs.uni-hannover.de

Soil profiles from Bavaria in southern Germany and from Chile were analysed for (129)I by accelerator mass spectrometry (AMS), for (127)I by inductively coupled plasma mass spectrometry (ICP-MS), and for (137)Cs by gamma-spectrometry. The mean deposition density of (137)Cs in soils from Bavaria was (41×1.5(±1)) kBq m(-2) (geometric mean and geometric standard deviation), originating mostly from the Chernobyl fall-out. The deposition density of (129)I in these soils was (109×1.5(±1)) mBq m(-2). The dominant sources of (129)I in Bavaria are, however, the reprocessing plants La Hague and Sellafield and not the Chernobyl fall-out. The (129)I/(127)I isotopic ratios of the Bavarian soils were between 10(-7) and 10(-10), i.e. 10(2)-10(5) times higher than the ratios observed for the samples from Chile. The (129)I integral deposition densities in Chile, Easter Island and Antarctica were between 0.3 mBq m(-2) and 2 mBq m(-2). In these soils, the observed (129)I/(127)I ratios were about 10(-12). The soils from Chile allow the determination of the (129)I fall-out from the atmospheric nuclear weapons explosions undisturbed from contaminations due to releases from reprocessing plants. An upper limit of the integral (129)I deposition density of the atmospheric nuclear weapons explosions on the Southern Hemisphere (27°S) is about 1 mBq m(-2). Finally, the dependence of the migration behaviour of (137)Cs, (127)I and of (129)I on the soil properties is discussed. It turns out that there is a distinctly different behaviour of (127)I, (129)I, and (137)Cs in the soils exhibiting different sorption mechanisms for old and recent iodine as well as for (137)Cs.

UI MeSH Term Description Entries
D007455 Iodine A nonmetallic element of the halogen group that is represented by the atomic symbol I, atomic number 53, and atomic weight of 126.90. It is a nutritionally essential element, especially important in thyroid hormone synthesis. In solution, it has anti-infective properties and is used topically. Iodine-127,Iodine 127
D007457 Iodine Radioisotopes Unstable isotopes of iodine that decay or disintegrate emitting radiation. I atoms with atomic weights 117-139, except I 127, are radioactive iodine isotopes. Radioisotopes, Iodine
D011834 Radiation Monitoring The observation, either continuously or at intervals, of the levels of radiation in a given area, generally for the purpose of assuring that they have not exceeded prescribed amounts or, in case of radiation already present in the area, assuring that the levels have returned to those meeting acceptable safety standards. Monitoring, Radiation
D011847 Radioactive Fallout The material that descends to the earth or water well beyond the site of a surface or subsurface nuclear explosion. (McGraw-Hill Dictionary of Chemical and Technical Terms, 4th ed) Fallout, Radioactive,Fallouts, Radioactive,Radioactive Fallouts
D002586 Cesium A member of the alkali metals. It has an atomic symbol Cs, atomic number 55, and atomic weight 132.91. Cesium has many industrial applications, including the construction of atomic clocks based on its atomic vibrational frequency. Caesium,Caesium-133,Cesium-133,Caesium 133,Cesium 133
D002588 Cesium Radioisotopes Unstable isotopes of cesium that decay or disintegrate emitting radiation. Cs atoms with atomic weights of 123, 125-132, and 134-145 are radioactive cesium isotopes. Radioisotopes, Cesium
D002677 Chile A country in southern South America, bordering the South Pacific Ocean, between Argentina and Peru.
D005858 Germany A country in central Europe, bordering the Baltic Sea and the North Sea, between the Netherlands and Poland, south of Denmark. The capital is Berlin.
D012990 Soil Pollutants, Radioactive Pollutants, present in soil, which exhibit radioactivity. Pollutants, Radioactive Soil,Radioactive Soil Pollutants
D013051 Spectrometry, Gamma Determination of the energy distribution of gamma rays emitted by nuclei. (McGraw-Hill Dictionary of Scientific and Technical Terms, 4th ed) Gamma Spectrophotometry,Gamma Spectrometry,Spectrophotometry, Gamma

Related Publications

A Daraoui, and R Michel, and M Gorny, and D Jakob, and R Sachse, and H-A Synal, and V Alfimov
June 2003, The Science of the total environment,
A Daraoui, and R Michel, and M Gorny, and D Jakob, and R Sachse, and H-A Synal, and V Alfimov
March 1999, The Science of the total environment,
A Daraoui, and R Michel, and M Gorny, and D Jakob, and R Sachse, and H-A Synal, and V Alfimov
January 2003, Journal of environmental radioactivity,
A Daraoui, and R Michel, and M Gorny, and D Jakob, and R Sachse, and H-A Synal, and V Alfimov
January 1976, Health physics,
A Daraoui, and R Michel, and M Gorny, and D Jakob, and R Sachse, and H-A Synal, and V Alfimov
April 2016, Journal of environmental radioactivity,
A Daraoui, and R Michel, and M Gorny, and D Jakob, and R Sachse, and H-A Synal, and V Alfimov
February 1959, Nature,
A Daraoui, and R Michel, and M Gorny, and D Jakob, and R Sachse, and H-A Synal, and V Alfimov
July 2000, Chemosphere,
A Daraoui, and R Michel, and M Gorny, and D Jakob, and R Sachse, and H-A Synal, and V Alfimov
March 1992, The Analyst,
A Daraoui, and R Michel, and M Gorny, and D Jakob, and R Sachse, and H-A Synal, and V Alfimov
January 1989, The British journal of radiology,
A Daraoui, and R Michel, and M Gorny, and D Jakob, and R Sachse, and H-A Synal, and V Alfimov
September 2013, Environmental science & technology,
Copied contents to your clipboard!