Interface control by homoepitaxial growth in pulsed laser deposited iron chalcogenide thin films. 2015

Sebastian Molatta, and Silvia Haindl, and Sascha Trommler, and Michael Schulze, and Sabine Wurmehl, and Ruben Hühne
Dresden High Magnetic Field Laboratory (HLD-EMFL), Helmholtz-Zentrum Dresden-Rossendorf, D-01314 Dresden, Germany.

Thin film growth of iron chalcogenides by pulsed laser deposition (PLD) is still a delicate issue in terms of simultaneous control of stoichiometry, texture, substrate/film interface properties, and superconducting properties. The high volatility of the constituents sharply limits optimal deposition temperatures to a narrow window and mainly challenges reproducibility for vacuum based methods. In this work we demonstrate the beneficial introduction of a semiconducting FeSe(1-x)Te(x) seed layer for subsequent homoepitaxial growth of superconducting FeSe(1-x)Te(x) thin film on MgO substrates. MgO is one of the most favorable substrates used in superconducting thin film applications, but the controlled growth of iron chalcogenide thin films on MgO has not yet been optimized and is the least understood. The large mismatch between the lattice constants of MgO and FeSe(1-x)Te(x) of about 11% results in thin films with a mixed texture, that prevents further accurate investigations of a correlation between structural and electrical properties of FeSe(1-x)Te(x). Here we present an effective way to significantly improve epitaxial growth of superconducting FeSe(1-x)Te(x) thin films with reproducible high critical temperatures (≥17 K) at reduced deposition temperatures (200 °C-320 °C) on MgO using PLD. This offers a broad scope of various applications.

UI MeSH Term Description Entries

Related Publications

Sebastian Molatta, and Silvia Haindl, and Sascha Trommler, and Michael Schulze, and Sabine Wurmehl, and Ruben Hühne
April 2019, Optics letters,
Sebastian Molatta, and Silvia Haindl, and Sascha Trommler, and Michael Schulze, and Sabine Wurmehl, and Ruben Hühne
January 2016, Scientific reports,
Sebastian Molatta, and Silvia Haindl, and Sascha Trommler, and Michael Schulze, and Sabine Wurmehl, and Ruben Hühne
May 2016, Scientific reports,
Sebastian Molatta, and Silvia Haindl, and Sascha Trommler, and Michael Schulze, and Sabine Wurmehl, and Ruben Hühne
May 2020, RSC advances,
Sebastian Molatta, and Silvia Haindl, and Sascha Trommler, and Michael Schulze, and Sabine Wurmehl, and Ruben Hühne
May 2019, Nanomaterials (Basel, Switzerland),
Sebastian Molatta, and Silvia Haindl, and Sascha Trommler, and Michael Schulze, and Sabine Wurmehl, and Ruben Hühne
October 2015, ACS applied materials & interfaces,
Sebastian Molatta, and Silvia Haindl, and Sascha Trommler, and Michael Schulze, and Sabine Wurmehl, and Ruben Hühne
October 2009, Biomaterials,
Sebastian Molatta, and Silvia Haindl, and Sascha Trommler, and Michael Schulze, and Sabine Wurmehl, and Ruben Hühne
June 1986, Applied optics,
Sebastian Molatta, and Silvia Haindl, and Sascha Trommler, and Michael Schulze, and Sabine Wurmehl, and Ruben Hühne
October 2006, Journal of microscopy,
Sebastian Molatta, and Silvia Haindl, and Sascha Trommler, and Michael Schulze, and Sabine Wurmehl, and Ruben Hühne
January 2020, International journal of bioprinting,
Copied contents to your clipboard!