Interaction of porphyrins and metalloporphyrins with nucleic acids. 1989

E J Gibbs, and R F Pasternack
Department of Chemistry, Goucher College, Towson, MD.

Differences in the interpretation of the details of the binding of porphyrins and metalloporphyrins to nucleic acids do exist, in part arising from the fact that different experimental techniques require different experimental conditions. For example, uv/vis absorption and CD spectroscopy use mumol/L and 10 to 100 mumol/L concentrations of drug and polymer respectively; whereas NMR uses mmol/l concentrations, increasing the likelihood of DNA aggregation. Differences in solvent conditions can have a profound effect on binding; changes in binding mode with changes in ionic strength have been observed for two of the porphyrins studied. At high levels of drug load the nucleic acid conformation may be changing and/or new modes of binding may become important. Thus, care must be taken when comparing data at different experimental conditions. At the same time that these various complexities for binding make comparison difficult it is precisely because of such complexities that these porphyrins are such sensitive probes of nucleic acid structure and dynamics. It may well be the diversity of binding of these porphyrins that will provide a variety of avenues for therapeutic strategies. It is certainly true that obtaining a complete binding picture for these porphyrins will require extended studies using a variety of techniques and experimental conditions.(ABSTRACT TRUNCATED AT 250 WORDS)

UI MeSH Term Description Entries
D008665 Metalloporphyrins Porphyrins which are combined with a metal ion. The metal is bound equally to all four nitrogen atoms of the pyrrole rings. They possess characteristic absorption spectra which can be utilized for identification or quantitative estimation of porphyrins and porphyrin-bound compounds. Metalloporphyrin
D009696 Nucleic Acids High molecular weight polymers containing a mixture of purine and pyrimidine nucleotides chained together by ribose or deoxyribose linkages. Nucleic Acid,Acid, Nucleic,Acids, Nucleic
D011166 Porphyrins A group of compounds containing the porphin structure, four pyrrole rings connected by methine bridges in a cyclic configuration to which a variety of side chains are attached. The nature of the side chain is indicated by a prefix, as uroporphyrin, hematoporphyrin, etc. The porphyrins, in combination with iron, form the heme component in biologically significant compounds such as hemoglobin and myoglobin. Porphyrin
D002417 Cattle Domesticated bovine animals of the genus Bos, usually kept on a farm or ranch and used for the production of meat or dairy products or for heavy labor. Beef Cow,Bos grunniens,Bos indicus,Bos indicus Cattle,Bos taurus,Cow,Cow, Domestic,Dairy Cow,Holstein Cow,Indicine Cattle,Taurine Cattle,Taurus Cattle,Yak,Zebu,Beef Cows,Bos indicus Cattles,Cattle, Bos indicus,Cattle, Indicine,Cattle, Taurine,Cattle, Taurus,Cattles, Bos indicus,Cattles, Indicine,Cattles, Taurine,Cattles, Taurus,Cow, Beef,Cow, Dairy,Cow, Holstein,Cows,Dairy Cows,Domestic Cow,Domestic Cows,Indicine Cattles,Taurine Cattles,Taurus Cattles,Yaks,Zebus
D000818 Animals Unicellular or multicellular, heterotrophic organisms, that have sensation and the power of voluntary movement. Under the older five kingdom paradigm, Animalia was one of the kingdoms. Under the modern three domain model, Animalia represents one of the many groups in the domain EUKARYOTA. Animal,Metazoa,Animalia

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