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Two-Step Spin-Crossover with Three Inequivalent FeII Sites in a Two-Dimensional Hofmann-Type Coordination Polymer. 2017
Yan Meng, and
Qing-Qing Sheng, and
Md Najbul Hoque, and
Yan-Cong Chen, and
Si-Guo Wu, and
Jiri Tucek, and
Radek Zboril, and
Tao Liu, and
Zhao-Ping Ni, and
Ming-Liang Tong
Key Laboratory of Bioinorganic and Synthetic Chemistry of Ministry of Education, School of Chemistry, Sun Yat-Sen University, Guangzhou, 510275, P. R. China.
An unprecedented two-step spin-crossover behavior with the sequence of γHS =1↔γHS =3/4↔γHS =1/4 was observed in two-dimensional Hofmann type coordination polymer [Fe(isoq)2 {Ag(CN)2 }2 ] (isoq=isoquinoline), which resulted from three crystallographically inequivalent FeII sites with distinct transition temperatures.
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