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Metal-Organic Framework-Stabilized CO2/Water Interfacial Route for Photocatalytic CO2 Conversion. 2017
Tian Luo, and
Jianling Zhang, and
Wei Li, and
Zhenhong He, and
Xiaofu Sun, and
Jinbiao Shi, and
Dan Shao, and
Bingxing Zhang, and
Xiuniang Tan, and
Buxing Han
Beijing National Laboratory for Molecular Sciences, CAS Key Laboratory of Colloid, Interface and Chemical Thermodynamics, Institute of Chemistry, Chinese Academy of Sciences, University of Chinese Academy of Sciences , Beijing 100190, P. R. China.
Here, we propose a CO2/water interfacial route for photocatalytic CO2 conversion by utilizing a metal-organic framework (MOF) as both an emulsifier and a catalyst. The CO2 reduction occurring at the CO2/water interface produces formate with remarkably enhanced efficiency as compared with that in conventional solvent. The route is efficient, facile, adjustable, and environmentally benign, which is applicable for the CO2 transformation photocatalyzed by different kinds of MOFs.
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