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Dual-catalytic decarbonylation of fatty acid methyl esters to form olefins. 2018
Megan E Fieser, and
Sydonie D Schimler, and
Lauren A Mitchell, and
Emily G Wilborn, and
Alex John, and
Levi T Hogan, and
Brooke Benson, and
Anne M LaPointe, and
William B Tolman
Department of Chemistry, Center for Sustainable Polymers, University of Minnesota, 207 Pleasant St. SE, Minneapolis, Minnesota 55455, USA.
The homogeneous dehydrative decarbonylation of fatty acid methyl esters (FAMEs) to form olefins is reported. In order to facilitate cleavage of the unactivated acyl C-O bond of the alkyl ester, a one pot dual-catalytic directing group strategy was developed through optimization of the individual transesterification and decarbonylation reaction steps.
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