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Photophysics of indole upon X-ray absorption. 2018
Thomas Kierspel, and
Cédric Bomme, and
Michele Di Fraia, and
Joss Wiese, and
Denis Anielski, and
Sadia Bari, and
Rebecca Boll, and
Benjamin Erk, and
Jens S Kienitz, and
Nele L M Müller, and
Daniel Rolles, and
Jens Viefhaus, and
Sebastian Trippel, and
Jochen Küpper
Center for Free-Electron Laser Science, Deutsches Elektronen-Synchrotron DESY, 22607 Hamburg, Germany. sebastian.trippel@cfel.de.
A photofragmentation study of gas-phase indole (C8H7N) upon single-photon ionization at a photon energy of 420 eV is presented. Indole was primarily inner-shell ionized at its nitrogen and carbon 1s orbitals. Electrons and ions were measured in coincidence by means of velocity map imaging. The angular relationship between ionic fragments is discussed along with the possibility to use the angle-resolved coincidence detection to perform experiments on molecules that are strongly oriented in their recoil-frame. The coincident measurement of electrons and ions revealed fragmentation-pathway-dependent electron spectra, linking the structural fragmentation dynamics to different electronic excitations. Evidence for photoelectron-impact self-ionization was observed.
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