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Structural evolution in a melt-quenched zeolitic imidazolate framework glass during heat-treatment. 2019
Jiayan Zhang, and
Louis Longley, and
Hao Liu, and
Christopher W Ashling, and
Philip A Chater, and
Kevin A Beyer, and
Karena W Chapman, and
Haizheng Tao, and
David A Keen, and
Thomas D Bennett, and
Yuanzheng Yue
State Key Laboratory of Silicate Materials for Architectures, Wuhan University of Technology, Wuhan 430070, China.
A pronounced enthalpy release occurs around 1.38Tg in the prototypical metal-organic framework glass formed from ZIF-4 [Zn(C3H3N2)2], but there is no sign for any crystallization (i.e., long-range ordering) taking place. The enthalpy release peak is attributed to pore collapse and structural densification.
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