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Ion-Pairing Assemblies Comprising Anion Complexes of π-Extended Anion-Responsive Molecules. 2019
Shinya Sugiura, and
Wakana Matsuda, and
Wanying Zhang, and
Shu Seki, and
Nobuhiro Yasuda, and
Hiromitsu Maeda
Department of Applied Chemistry, College of Life Sciences , Ritsumeikan University , Kusatsu 525-8577 , Japan.
Anion-responsive molecules comprising phenanthropyrrole rings were synthesized by oxidative coupling. Spectroscopic and theoretical examinations revealed the effects of the π-extended structures. In the solid state as ion-pairing assemblies, Cl- complexes of π-extended derivatives formed stacked structures composed of Cl- complexes themselves and those formed with countercations using extended π-moieties. Aliphatic anion-responsive molecules and their Cl- complexes, as ion pairs with the triazatriangulenium cation, provided hexagonal columnar structures with liquid-crystalline mesophases.
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