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ROMPI-CDSA: ring-opening metathesis polymerization-induced crystallization-driven self-assembly of metallo-block copolymers. 2019
Ye Sha, and
Md Anisur Rahman, and
Tianyu Zhu, and
Yujin Cha, and
C Wayne McAlister, and
Chuanbing Tang
Department of Chemistry and Biochemistry , University of South Carolina , Columbia , South Carolina 29208 , USA . Email: tang4@mailbox.sc.edu.
Polymerization-induced self-assembly (PISA) and crystallization-driven self-assembly (CDSA) are among the most prevailing methods for block copolymer self-assembly. Taking the merits of scalability of PISA and dimension control of CDSA, we report one-pot synchronous PISA and CDSA via ring-opening metathesis polymerization (ROMP) to prepare nano-objects based on a crystalline poly(ruthenocene) motif. We denote this self-assembly methodology as ROMPI-CDSA to enable a simple, yet robust approach for the preparation of functional nanomaterials.
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