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High Adsorption Capacity and Selectivity of SO2 over CO2 in a Metal-Organic Framework. 2021
Ya Ling Fan, and
Hui Ping Zhang, and
Meng Jia Yin, and
Rajamani Krishna, and
Xue Feng Feng, and
Li Wang, and
Ming Biao Luo, and
Feng Luo
School of Biology, Chemistry and Material Science, East China University of Technology, Nanchang, Jiangxi 344000, China.
Herein, we report a new metal-organic framework (MOF), namely, ECUT-77, which is built on rod-shaped secondary building units, showing a high Brunauer-Emmett-Teller surface area of 760.3 cm2/g, a pore volume of 0.4 cm3/g, and an aperture of about 1 nm. This MOF enables both high SO2 adsorption capacity up to 8.0 mmol/g at 0.92 bar and room temperature and a high SO2/CO2 selectivity of 44, resulting in excellent SO2 separation upon a ECUT-77 column from a SO2/CO2 mixture containing 2000 ppm of SO2.
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