Source noise suppression in attosecond transient absorption spectroscopy by edge-pixel referencing. 2021

Romain Géneaux, and Hung-Tzu Chang, and Adam M Schwartzberg, and Hugo J B Marroux

Attosecond transient absorption spectroscopy (ATAS) is used to observe photoexcited dynamics with outstanding time resolution. The main experimental challenge of this technique is that high-harmonic generation sources show significant instabilities, resulting in sub-par sensitivity when compared to other techniques. This paper proposes edge-pixel referencing as a means to suppress this noise. Two approaches are introduced: the first is deterministic and uses a correlation analysis, while the second relies on singular value decomposition. Each method is demonstrated and quantified on a noisy measurement taken on WS2 and results in a fivefold increase in sensitivity. The combination of the two methods ensures the fidelity of the procedure and can be implemented on live data collection but also on existing datasets. The results show that edge-referencing methods bring the sensitivity of ATAS near the detector noise floor. An implementation of the post-processing code is provided to the reader.

UI MeSH Term Description Entries

Related Publications

Romain Géneaux, and Hung-Tzu Chang, and Adam M Schwartzberg, and Hugo J B Marroux
March 2020, The Journal of chemical physics,
Romain Géneaux, and Hung-Tzu Chang, and Adam M Schwartzberg, and Hugo J B Marroux
October 2019, Optics letters,
Romain Géneaux, and Hung-Tzu Chang, and Adam M Schwartzberg, and Hugo J B Marroux
September 2021, Physical review letters,
Romain Géneaux, and Hung-Tzu Chang, and Adam M Schwartzberg, and Hugo J B Marroux
July 2018, Physical review letters,
Romain Géneaux, and Hung-Tzu Chang, and Adam M Schwartzberg, and Hugo J B Marroux
July 2019, Science (New York, N.Y.),
Romain Géneaux, and Hung-Tzu Chang, and Adam M Schwartzberg, and Hugo J B Marroux
February 2020, Physical chemistry chemical physics : PCCP,
Romain Géneaux, and Hung-Tzu Chang, and Adam M Schwartzberg, and Hugo J B Marroux
March 2022, The Journal of chemical physics,
Romain Géneaux, and Hung-Tzu Chang, and Adam M Schwartzberg, and Hugo J B Marroux
May 2021, Faraday discussions,
Romain Géneaux, and Hung-Tzu Chang, and Adam M Schwartzberg, and Hugo J B Marroux
June 2021, The Journal of chemical physics,
Romain Géneaux, and Hung-Tzu Chang, and Adam M Schwartzberg, and Hugo J B Marroux
March 2011, Physical review letters,
Copied contents to your clipboard!