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Chitin/Metal-Organic Framework Composites as Wide-Range Adsorbent. 2021
Gabriel I Tovar Jimenez, and
Ainara Valverde, and
Cristian Mendes-Felipe, and
Stefan Wuttke, and
Arkaitz Fidalgo-Marijuan, and
Edurne S Larrea, and
Luis Lezama, and
Fangyuan Zheng, and
Javier Reguera, and
Senentxu Lanceros-Méndez, and
María I Arriortua, and
Guillermo Copello, and
Roberto Fernández de Luis
Facultad de Farmacia y Bioquímica, Departamento de Química Analítica y Fisicoquímica, Universidad de Buenos Aires (UBA), Junín 956, C1113AAD, Buenos Aires, Argentina.
Composites based on chitin (CH) biopolymer and metal-organic framework (MOF) microporous nanoparticles have been developed as broad-scope pollutant absorbent. Detailed characterization of the CH/MOF composites revealed that the MOF nanoparticles interacted through electrostatic forces with the CH matrix, inducing compartmentalization of the CH macropores that led to an overall surface area increase in the composites. This created a micro-, meso-, and macroporous structure that efficiently retained pollutants with a broad spectrum of different chemical natures, charges, and sizes. The unique prospect of this approach is the combination of the chemical diversity of MOFs with the simple processability and biocompatibility of CH that opens application fields beyond water remediation.
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