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Shedding light on the energy applications of emerging 2D hybrid organic-inorganic halide perovskites. 2022

Neng Li, and Yufei Yang, and Zuhao Shi, and Zhigao Lan, and Arramel Arramel, and Peng Zhang, and Wee-Jun Ong, and Jizhou Jiang, and Jianfeng Lu
State Key Laboratory of Silicate Materials for Architecture, Wuhan University of Technology, Wuhan 430070, China.

Unique performance of the hybrid organic-inorganic halide perovskites (HOIPs) has attracted great attention because of their continuous exploration and breakthrough in a multitude of energy-related applications. However, the instability and lead-induced toxicity that arise in bulk perovskites are the two major challenges that impede their future commercialization process. To find a solution, a series of two-dimensional HOIPs (2D HOIPs) are investigated to prolong the device lifetime with highly efficient photoelectric conversion and energy storage. Herein, the recent advances of 2D HOIPs and their structural derivatives for the energy realms are summarized and discussed. The basic understanding of crystal structures, physicochemical properties, and growth mechanisms is presented. In addition, the current challenges and future directions to provide a roadmap for the development of next generation 2D HOIPs are prospected.

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