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Phosphorus-Doped Graphene Electrocatalysts for Oxygen Reduction Reaction. 2022

Xinxing Zhan, and Xin Tong, and Manqi Gu, and Juan Tian, and Zijian Gao, and Liying Ma, and Yadian Xie, and Zhangsen Chen, and Hariprasad Ranganathan, and Gaixia Zhang, and Shuhui Sun
School of Chemistry and Material Science, Guizhou Normal University, Guiyang 550001, China.

Developing cheap and earth-abundant electrocatalysts with high activity and stability for oxygen reduction reactions (ORRs) is highly desired for the commercial implementation of fuel cells and metal-air batteries. Tremendous efforts have been made on doped-graphene catalysts. However, the progress of phosphorus-doped graphene (P-graphene) for ORRs has rarely been summarized until now. This review focuses on the recent development of P-graphene-based materials, including the various synthesis methods, ORR performance, and ORR mechanism. The applications of single phosphorus atom-doped graphene, phosphorus, nitrogen-codoped graphene (P, N-graphene), as well as phosphorus, multi-atoms codoped graphene (P, X-graphene) as catalysts, supporting materials, and coating materials for ORR are discussed thoroughly. Additionally, the current issues and perspectives for the development of P-graphene materials are proposed.

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