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2D Covalent Organic Frameworks Toward Efficient Photocatalytic Hydrogen Evolution. 2022

Yang Li, and Xiaoyu Song, and Guang Zhang, and Lei Wang, and Yi Liu, and Weihua Chen, and Long Chen
Shenzhen Key Laboratory of Polymer Science and Technology, Guangdong Research Center for Interfacial Engineering of Functional Materials, College of Materials Science and Engineering, Shenzhen University, Shenzhen, 518060, P. R. China.

Efficiently producing clean energy is of great importance for sustainable development of the environment. Solar-driven water splitting for H2 evolution has an important role among the renewable energy technologies. Developing high-performance and cost-effective photocatalysts is still a critical task before practical application. 2D Covalent organic frameworks (COFs) as photocatalysts have recently attracted widespread interest thanks to their tunable optical bandgaps, tailor-made functionality, excellent crystallinity, high specific surface area, and good photo- and chemical stability. This Review focuses on the representative progress and remaining challenges in 2D COF-based photocatalysts for hydrogen evolution.

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