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A viologen-functionalized metal-organic framework for efficient CO2 photoreduction reaction. 2022
Tong Wang, and
Lei Zhang, and
Jiang Liu, and
Xiao-Xin Li, and
Lin Yuan, and
Shun-Li Li, and
Ya-Qian Lan
Jiangsu Collaborative Innovation Centre of Biomedical Functional Materials, Jiangsu Key Laboratory of New Power Batteries, School of Chemistry and Materials Science, Nanjing Normal University, Nanjing 210023, P. R. China. liuj@njnu.edu.cn.
Here, a viologen-functionalized metal-organic framework (MOF), MIL-125-RV2+, was obtained by modification of MIL-125-NH2 with viologen molecules. MIL-125-RV2+, the first viologen-based MOF for photocatalytic CO2RR, exhibited excellent photocatalytic activity and high selectivity for HCOO-. The strategy of using photo-responsive color-changing organics to functionalize the MOF is significant for achieving efficient CO2RR.
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