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Femtosecond Rotational Dynamics of D_{2} Molecules in Superfluid Helium Nanodroplets. 2022
Junjie Qiang, and
Lianrong Zhou, and
Peifen Lu, and
Kang Lin, and
Yongzhe Ma, and
Shengzhe Pan, and
Chenxu Lu, and
Wenyu Jiang, and
Fenghao Sun, and
Wenbin Zhang, and
Hui Li, and
Xiaochun Gong, and
Ilya Sh Averbukh, and
Yehiam Prior, and
Constant A Schouder, and
Henrik Stapelfeldt, and
Igor N Cherepanov, and
Mikhail Lemeshko, and
Wolfgang Jäger, and
Jian Wu
State Key Laboratory of Precision Spectroscopy, East China Normal University, Shanghai 200241, China.
Rotational dynamics of D_{2} molecules inside helium nanodroplets is induced by a moderately intense femtosecond pump pulse and measured as a function of time by recording the yield of HeD^{+} ions, created through strong-field dissociative ionization with a delayed femtosecond probe pulse. The yield oscillates with a period of 185 fs, reflecting field-free rotational wave packet dynamics, and the oscillation persists for more than 500 periods. Within the experimental uncertainty, the rotational constant B_{He} of the in-droplet D_{2} molecule, determined by Fourier analysis, is the same as B_{gas} for an isolated D_{2} molecule. Our observations show that the D_{2} molecules inside helium nanodroplets essentially rotate as free D_{2} molecules.
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