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An ato-topology metal-organic framework with large C2H2 adsorption and C2H2/CO2 separation capacity. 2022
Ting Wang, and
Zhi-Jie Jiang, and
Ying Wang, and
Rong-Jia Wei, and
Heng Zeng, and
Weigang Lu, and
Dan Li
College of Chemistry and Materials Science, and Guangdong Provincial Key Laboratory of Functional Supramolecular Coordination Materials and Applications, Jinan University, Guangzhou 510632, P. R. China. zengheng90@163.com.
The efficient separation of C2H2/CO2 is challenging and energy intensive due to their similar molecular shapes and kinetic diameters. Here we report an ato-topology metal-organic framework (JNU-7a) with a specific surface area of 2046 cm2 g-1 and open-metal-site density of 2.05 mmol cm-3, resulting in a large C2H2 adsorption capacity of (176 cm3 g-1) and high C2H2/CO2 adsorption selectivity (6.2).
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