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Carrier envelope phase sensitivity of photoelectron circular dichroism. 2023
Václav Hanus, and
Sarayoo Kangaparambil, and
Martin Richter, and
Lukas Haßfurth, and
Martin Dorner-Kirchner, and
Gerhard G Paulus, and
Xinhua Xie, and
Andrius Baltuška, and
Stefanie Gräfe, and
Markus Zeiler
Photonics Institute, Technische Universität Wien, 1040 Vienna, Austria. hanus.vaclav@wigner.hu.
We report on a combined experimental and numerical study of photoelectron circular dichroism (PECD) induced by intense few-cycle laser pulses, using methyloxirane as the molecular example. Our experiments reveal a remarkably pronounced sensitivity of the PECD strength of double-ionization on the carrier-envelope phase (CEP) of the laser pulses. By comparison to the simulations, which reproduce the measured CEP-dependence for specific orientations of the molecules in the lab frame, we attribute the origin of the observed CEP-dependence of PECD to the CEP-induced modulation of ionization from different areas of the wave functions of three dominant orbitals.
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