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BiVO4-Deposited MIL-101-NH2 for Efficient Photocatalytic Elimination of Cr(VI). 2023
Huiwen Sun, and
Qihang Dai, and
Ju Liu, and
Tiantian Zhou, and
Muhua Chen, and
Zhengchun Cai, and
Xinbao Zhu, and
Bo Fu
Jiangsu Co-Innovation Center of Efficient Processing and Utilization of Forest Resources, Jiangsu Provincial Key Lab for the Chemistry and Utilization of Agro-Forest Biomass, College of Chemical Engineering, Nanjing Forestry University, Nanjing 210037, China.
In this study, a flower-like BiVO4/MIL-101-NH2 composite is synthesized by a facile and surfactant-free process. The -COO--Bi3+ ionic bond construction was conductive to enhance the interface affinity between BiVO4 and MIL-101-NH2. Due to the highly efficient light capture and sufficient electron traps induced by oxygen vacancies and the formation of a heterostructure, the improved separation and transportation rates of charge carriers are realized. In addition, the MIL-101-NH2/BiVO4 composite is favorable for Cr(VI) photocatalytic removal (91.2%). Moreover, FNBV-3 (Fe/Bi = 0.25) also exhibited an excellent reusability after five cycles.
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