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Stepwise assembly of heterometallic, heteroleptic "triblock Janus-type" metal-organic polyhedra. 2023
Cornelia von Baeckmann, and
Sara Ruiz-Relaño, and
Inhar Imaz, and
Marcel Handke, and
Judith Juanhuix, and
Felipe Gándara, and
Arnau Carné-Sanchez, and
Daniel Maspoch
Catalan Institute of Nanoscience and Nanotechnology (ICN2), CSIC, and The Barcelona Institute of Science and Technology, Campus UAB, Bellaterra, Barcelona 08193, Spain. arnau.carne@icn2.cat.
Increasing the chemical complexity of metal-organic cages (MOCs) or polyhedra (MOPs) demands control over the simultaneous organization of diverse organic linkers and metal ions into discrete caged structures. Herein, we show that a pre-assembled complex of the archetypical cuboctahedral MOP can be used as a template to replicate such caged structure, one having a "triblock Janus-type" configuration that is both heterometallic and heteroleptic.
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