Water purification using thin membranes at high pressures through adsorption and size exclusion is the widely used mechanism due to its simplicity and enhanced efficiency compared to other traditional water purification methods. Aerogels have the potential to replace conventional thin membranes considering their unmatched adsorption/absorption capacity and higher water flux due to their unique highly porous (99 %) 3D structure, ultra-low density (~1.1 to 500 mg/cm3), and very high surface area. The availability of a large number of functional groups, surface tunability, hydrophilicity, tensile strength and flexibility of nanocellulose (NC) makes it a potential candidate for aerogel preparation. This review discusses the preparation and employment of NC-based aerogels in the removal of dyes, metal ions and oils/organic solvents. It also offers recent updates on the effect of various parameters that enhance its adsorption/absorption performance. The future perspectives of NC aerogels and their performance with the emerging materials chitosan and graphene oxide are also compared.