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Lead zirconate titanate ceramics with aligned crystallite grains. 2023
Jinglei Li, and
Wanbo Qu, and
John Daniels, and
Haijun Wu, and
Linjing Liu, and
Jie Wu, and
Mingwen Wang, and
Stefano Checchia, and
Shuai Yang, and
Haobin Lei, and
Rui Lv, and
Yang Zhang, and
Danyang Wang, and
Xuexin Li, and
Xiangdong Ding, and
Jun Sun, and
Zhuo Xu, and
Yunfei Chang, and
Shujun Zhang, and
Fei Li
Electronic Materials Research Laboratory (Key Lab of Education Ministry), State Key Laboratory for Mechanical Behavior of Materials and School of Electronic and Information Engineering, Xi'an Jiaotong University, Xi'an 710049, China.
The piezoelectric properties of lead zirconate titanate [Pb(Zr,Ti)O3 or PZT] ceramics could be enhanced by fabricating textured ceramics that would align the crystal grains along specific orientations. We present a seed-passivated texturing process to fabricate textured PZT ceramics by using newly developed Ba(Zr,Ti)O3 microplatelet templates. This process not only ensures the template-induced grain growth in titanium-rich PZT layers but also facilitates desired composition through interlayer diffusion of zirconium and titanium. We successfully prepared textured PZT ceramics with outstanding properties, including Curie temperatures of 360°C, piezoelectric coefficients d33 of 760 picocoulombs per newton and g33 of 100 millivolt meters per newton, and electromechanical couplings k33 of 0.85. This study addresses the challenge of fabricating textured rhombohedral PZT ceramics by suppressing the otherwise severe chemical reaction between PZT powder and titanate templates.
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