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Cobalt porphyrin-based hypercrosslinked ionic polymers as biomimetic nanoreactors for CO2 conversion to cyclic carbonates. 2024
School of Chemical Engineering and Light Industry, Guangdong University of Technology, Guangzhou 510006, China. luorch@gdut.edu.cn.
A simple and low-cost approach to construct one type of cobalt porphyrin-based hypercrosslinked ionic polymer with high specific surface areas, densely located ionic groups and highly dispersed cobalt sites has been demonstrated, which act as bifunctional catalysts for the solvent-additive-free conversion of CO2 into cyclic carbonates with outstanding biomimetic catalytic performance and good recyclability.
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