Complex reaction pathway of aryl beta-xyloside degradation by beta-xylanase of Cryptococcus albidus. 1980

P Biely, and M Vrsanská, and Z Krátký

The extracellular endo-1,4-beta-xylanase of the yeast Cryptococcus albidus catalyzes degradation of aryl beta-xylosides by other reactions than simple hydrolytic cleavage. Liberation of phenol or p-nitrophenol from the corresponding beta-xylosides is accompanied by formation of xylose oligosaccharides and only small amounts of xylose. With the aid of phenyl beta-[U-14C]xyloside synthesized from [U-14C]xylose, it was established that the reaction followed a complex pattern with the rate of phenyl beta-xyloside digestion and appearance of various products varying markedly with time. The reaction involves multiple transglycosylic reaction leading first to phenyl glycosides of xylooligosaccharides, which are subsequently hydrolyzed mainly to xylobiose and xylotriose. At concentrations of phenyl beta-xyloside lower than 100 mM the reaction exhibited a significant lag phase, which was followed by period during which the rate of the degradation of the substrate could be determined. The rate showed a strong sigmoidal dependence on phenyl-beta-xyloside concentration. The lag phase could be eliminated and the initial rate accelerated by addition of xylose oligosaccharides, which are hydrolyzed by beta-xylanase. After disappearance of the added oligosaccharides, the reaction transitionally ceased and then resumed again at a rate comparable to the control without added oligosaccharides. It is proposed that beta-xylanase utilizes for degradation of phenyl beta-xyloside two reaction pathways differing in the nature of glycosyl donors.

UI MeSH Term Description Entries
D007553 Isotope Labeling Techniques for labeling a substance with a stable or radioactive isotope. It is not used for articles involving labeled substances unless the methods of labeling are substantively discussed. Tracers that may be labeled include chemical substances, cells, or microorganisms. Isotope Labeling, Stable,Isotope-Coded Affinity Tagging,Isotopically-Coded Affinity Tagging,Affinity Tagging, Isotope-Coded,Affinity Tagging, Isotopically-Coded,Isotope Coded Affinity Tagging,Labeling, Isotope,Labeling, Stable Isotope,Stable Isotope Labeling,Tagging, Isotope-Coded Affinity,Tagging, Isotopically-Coded Affinity
D007700 Kinetics The rate dynamics in chemical or physical systems.
D002250 Carbon Radioisotopes Unstable isotopes of carbon that decay or disintegrate emitting radiation. C atoms with atomic weights 10, 11, and 14-16 are radioactive carbon isotopes. Radioisotopes, Carbon
D003454 Cryptococcus A mitosporic Tremellales fungal genus whose species usually have a capsule and do not form pseudomycellium. Teleomorphs include Filobasidiella and Fidobasidium. Torula
D006026 Glycoside Hydrolases Any member of the class of enzymes that catalyze the cleavage of the glycosidic linkage of glycosides and the addition of water to the resulting molecules. Endoglycosidase,Exoglycosidase,Glycohydrolase,Glycosidase,Glycosidases,Glycoside Hydrolase,Endoglycosidases,Exoglycosidases,Glycohydrolases,Hydrolase, Glycoside,Hydrolases, Glycoside
D006027 Glycosides Any compound that contains a constituent sugar, in which the hydroxyl group attached to the first carbon is substituted by an alcoholic, phenolic, or other group. They are named specifically for the sugar contained, such as glucoside (glucose), pentoside (pentose), fructoside (fructose), etc. Upon hydrolysis, a sugar and nonsugar component (aglycone) are formed. (From Dorland, 28th ed; From Miall's Dictionary of Chemistry, 5th ed) Glycoside
D013379 Substrate Specificity A characteristic feature of enzyme activity in relation to the kind of substrate on which the enzyme or catalytic molecule reacts. Specificities, Substrate,Specificity, Substrate,Substrate Specificities
D014994 Xylose D-Xylose,D Xylose
D043364 Endo-1,4-beta Xylanases Enzymes which catalyze the endohydrolysis of 1,4-beta-D-xylosidic linkages in XYLANS. Endo-1,4-beta-Xylanase,1,4-beta-D-Xylanohydrolase,Beta-1-4-Endoxylanase,Endo-1,4-Xylanase II,Endo-1,4-beta-Xylanase II,Endoxylanase,Xylanase A,Xylanase B,Xylanase C,Xylanase D,Xylanase J,Xylanase Y,Xylanase Z,beta Xylanase,1,4 beta D Xylanohydrolase,Beta 1 4 Endoxylanase,Endo 1,4 Xylanase II,Endo 1,4 beta Xylanase,Endo 1,4 beta Xylanase II,Endo 1,4 beta Xylanases,Xylanase, beta,Xylanases, Endo-1,4-beta

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