Use of narrow-bore high-performance liquid chromatography-diode array detection for the analysis of intermediates of the biological degradation of 2,4,6-trinitrotoluene. 1995

F Ahmad, and D J Roberts
Department of Civil and Environmental Engineering, University of Houston, TX.

A single method was developed for the separation and quantitation of hexahydro-1,3,5-trinitro-1,3,5-triazine, 2,4,6-trinitrotoluene (TNT), and most of the known and suspected biodegradation intermediates of TNT by RP-HPLC and diode array detection. The known biodegradation intermediates of TNT analyzed were 2-amino-4,6-dinitrotoluene, 4-amino-2,6-dinitrotoluene, 2,6-diamino-4-nitrotoluene, 2,4-diamino-6-nitrotoluene, 2,4,6-triaminotoluene, 2,2',6,6'-tetranitro-4,4'-azoxytoluene, and 4,4',6,6'-tetranitro-2,2'-azoxytoluene. The suspected biodegradation intermediates of TNT included 1,2,3-benzenetriol (pyrogallol), 1,3,5-benzenetriol (phloroglucinol), 2-methyl-1,3,5-benzenetriol (methyl phloroglucinol) and 4-methylphenol (p-cresol). Mobile phases consisting of aqueous buffers adjusted to three different pH values in a gradient with acetonitrile were examined for their efficiency in separating the intermediate compounds and for the minimization of speciation of the ionizable intermediates (e.g. 2,4,6-triaminotoluene). A final aqueous buffer pH of 3.2 was selected to minimize the interference to the separation caused by 2,4,6-triaminotoluene speciation. Solvent consumption was minimized by the use of a narrow-bore column. All of the known reduction products as well as p-cresol and methyl phloroglucinol were identified in culture supernatants from TNT-degrading cultures while pyrogallol and phloroglucinol were not.

UI MeSH Term Description Entries
D002851 Chromatography, High Pressure Liquid Liquid chromatographic techniques which feature high inlet pressures, high sensitivity, and high speed. Chromatography, High Performance Liquid,Chromatography, High Speed Liquid,Chromatography, Liquid, High Pressure,HPLC,High Performance Liquid Chromatography,High-Performance Liquid Chromatography,UPLC,Ultra Performance Liquid Chromatography,Chromatography, High-Performance Liquid,High-Performance Liquid Chromatographies,Liquid Chromatography, High-Performance
D006863 Hydrogen-Ion Concentration The normality of a solution with respect to HYDROGEN ions; H+. It is related to acidity measurements in most cases by pH pH,Concentration, Hydrogen-Ion,Concentrations, Hydrogen-Ion,Hydrogen Ion Concentration,Hydrogen-Ion Concentrations
D001673 Biodegradation, Environmental Elimination of ENVIRONMENTAL POLLUTANTS; PESTICIDES and other waste using living organisms, usually involving intervention of environmental or sanitation engineers. Bioremediation,Phytoremediation,Natural Attenuation, Pollution,Environmental Biodegradation,Pollution Natural Attenuation
D013057 Spectrum Analysis The measurement of the amplitude of the components of a complex waveform throughout the frequency range of the waveform. (McGraw-Hill Dictionary of Scientific and Technical Terms, 6th ed) Spectroscopy,Analysis, Spectrum,Spectrometry
D014303 Trinitrotoluene A 2,4,6-trinitrotoluene, which is an explosive chemical that can cause skin irritation and other toxic consequences. TNT,2,4,6-Trinitrotoluene
D014867 Water A clear, odorless, tasteless liquid that is essential for most animal and plant life and is an excellent solvent for many substances. The chemical formula is hydrogen oxide (H2O). (McGraw-Hill Dictionary of Scientific and Technical Terms, 4th ed) Hydrogen Oxide

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