[Action of chlorphentermine on the hydrolysis of phosphatidyl choline by phospholipase A2 (author's transl)]. 1977

R Gräbner

OBJECTIVE The anorectic drug chlorphentermine (Chlph) has been reported to cause lipoidosis-like cellular alterations in many organs, especially in lungs. A weak inflammation has been observed during the first week of daily application. After that time a pronounced foam cell production with many lamellated inclusion bodies in the cell occurs. It has been supposed that this action is caused by an inhibition of phospholipid-degradation due to an association between the drug and phospholipids. To substantiate this mechanism an in vitro study a bout the action of Chlph on the hydrolysis of phosphytidyl choline (PC) by phospholipase A2 (bee venom) was undertaken. METHODS Pur PC was obtained by column chromatography of egg lecithin. PC was used in two physical states. Handshaken liposomes are used as a model of the lamellated inclusion bodies of drug- induced phospholipidosis. The kinetic analysis was carried out on single bilayered liposomes obtained by injection of an ethanolic PC-solution into 0.16 M KCl. Purified bee venom was used as enzyme source. Usually the drug was added before the initiation of the enzyme reaction. In some cases Chlph was added after starting the hydrolysis by phospholipase for a detailed characterization of the type of interaction between Chlph and PC. The velocity of the enzyme reaction was measured by pH- stat titration and was expressed as mM H+-release per min. RESULTS Two phases of Chlph-action are observed. A time limited stimulation of hydrolysis occurs immediatly after addition of the drug. The enzyme reaction is inhibited after the disappearence of this activation. This inhibition is independent of the physical state of the substrate and is very pronounced at equimolar mixtures of Chlph and PC (88 per cent inhibition in handshaken liposomes; 78 per cent inhibition in single bilayered liposomes). At inhibitor concentrations below 10 mol per cent the hydrolysis is not affected. By kinetic analysis it was found that the inhibitory action is due to an association between the inhibitor and the substrate. The Lineweaver-Burk- and Dixon-replots show a series of curves characteristic for this type of interaction (concave shape; no common intersections, situated in the 2nd quadrant). The intermediate stimulation of the substrate hydrolysis occurs only during the reaction of Chlph with PC. This is concluded from the following observations: The duration of activation is proportional to the inhibitor concentration as well as to the substrate concentration, i.e. it is proportional to the concentration of both reactants. The activation does not occur if the enzyme reaction is started some time after mixing inhibitor and substrate, i.e. after finishing the reaction. The results are discussed in relation to the in vivo action of Chlph.

UI MeSH Term Description Entries
D007700 Kinetics The rate dynamics in chemical or physical systems.
D008081 Liposomes Artificial, single or multilaminar vesicles (made from lecithins or other lipids) that are used for the delivery of a variety of biological molecules or molecular complexes to cells, for example, drug delivery and gene transfer. They are also used to study membranes and membrane proteins. Niosomes,Transferosomes,Ultradeformable Liposomes,Liposomes, Ultra-deformable,Liposome,Liposome, Ultra-deformable,Liposome, Ultradeformable,Liposomes, Ultra deformable,Liposomes, Ultradeformable,Niosome,Transferosome,Ultra-deformable Liposome,Ultra-deformable Liposomes,Ultradeformable Liposome
D010645 Phentermine A central nervous system stimulant and sympathomimetic with actions and uses similar to those of DEXTROAMPHETAMINE. It has been used most frequently in the treatment of obesity. Adipex-P,Duromine,Ionamine,Phentermine Hydrochloride,Adipex P,AdipexP,Hydrochloride, Phentermine
D010713 Phosphatidylcholines Derivatives of PHOSPHATIDIC ACIDS in which the phosphoric acid is bound in ester linkage to a CHOLINE moiety. Choline Phosphoglycerides,Choline Glycerophospholipids,Phosphatidyl Choline,Phosphatidyl Cholines,Phosphatidylcholine,Choline, Phosphatidyl,Cholines, Phosphatidyl,Glycerophospholipids, Choline,Phosphoglycerides, Choline
D010740 Phospholipases A class of enzymes that catalyze the hydrolysis of phosphoglycerides or glycerophosphatidates. EC 3.1.-. Lecithinases,Lecithinase,Phospholipase
D002745 Chlorphentermine A sympathomimetic agent that was formerly used as an anorectic. It has properties similar to those of DEXTROAMPHETAMINE. It has been implicated in lipid storage disorders and pulmonary hypertension. (From Martindale, The Extra Pharmacopoeia, 30th ed, p1223) Avipron,Chlorphentermine Hydrochloride,Desopimon,Pre-Sate,Hydrochloride, Chlorphentermine
D000818 Animals Unicellular or multicellular, heterotrophic organisms, that have sensation and the power of voluntary movement. Under the older five kingdom paradigm, Animalia was one of the kingdoms. Under the modern three domain model, Animalia represents one of the many groups in the domain EUKARYOTA. Animal,Metazoa,Animalia
D001516 Bees Insect members of the superfamily Apoidea, found almost everywhere, particularly on flowers. About 3500 species occur in North America. They differ from most WASPS in that their young are fed honey and pollen rather than animal food. Apidae,Apis,Apis mellifera,Apis mellifica,European Honey Bee,Honey Bee Drone,Bee,Bee, European Honey,Drone, Honey Bee,European Honey Bees,Honey Bee Drones,Honey Bee, European
D014688 Venoms Poisonous animal secretions forming fluid mixtures of many different enzymes, toxins, and other substances. These substances are produced in specialized glands and secreted through specialized delivery systems (nematocysts, spines, fangs, etc.) for disabling prey or predator. Venom

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