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Ring-closing olefin metathesis for the synthesis of benzene derivatives. 2006
Kazuhiro Yoshida, and
Fumihiro Kawagoe, and
Noriyuki Iwadate, and
Hidetoshi Takahashi, and
Tsuneo Imamoto
Department of Chemistry, Faculty of Science, Chiba University, Yayoi-cho, Inage-ku, Chiba 263-8522, Japan. kyoshida@faculty.chiba-u.jp
Benzene derivatives were synthesized in excellent yield from 1,4,7-trien-3-ols by tandem ruthenium-catalyzed ring-closing olefin metathesis (RCM)/dehydration. The method was extended to the tandem RCM/oxidation process to obtain phenol and aniline derivatives. This method displays many advantages over aromatic-substitution-based classical routes.
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