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Nitrate radicals and biogenic volatile organic compounds: oxidation, mechanisms, and organic aerosol. 2017
Nga Lee Ng, and
Steven S Brown, and
Alexander T Archibald, and
Elliot Atlas, and
Ronald C Cohen, and
John N Crowley, and
Douglas A Day, and
Neil M Donahue, and
Juliane L Fry, and
Hendrik Fuchs, and
Robert J Griffin, and
Marcelo I Guzman, and
Hartmut Herrmann, and
Alma Hodzic, and
Yoshiteru Iinuma, and
José L Jimenez, and
Astrid Kiendler-Scharr, and
Ben H Lee, and
Deborah J Luecken, and
Jingqiu Mao, and
Robert McLaren, and
Anke Mutzel, and
Hans D Osthoff, and
Bin Ouyang, and
Benedicte Picquet-Varrault, and
Ulrich Platt, and
Havala O T Pye, and
Yinon Rudich, and
Rebecca H Schwantes, and
Manabu Shiraiwa, and
Jochen Stutz, and
Joel A Thornton, and
Andreas Tilgner, and
Brent J Williams, and
Rahul A Zaveri
School of Chemical and Biomolecular Engineering, Georgia Institute of Technology, Atlanta, GA, USA.
Oxidation of biogenic volatile organic compounds (BVOC) by the nitrate radical (NO3) represents one of the important interactions between anthropogenic emissions related to combustion and natural emissions from the biosphere. This interaction has been recognized for more than 3 decades, during which time a large body of research has emerged from laboratory, field, and modeling studies. NO3-BVOC reactions influence air quality, climate and visibility through regional and global budgets for reactive nitrogen (particularly organic nitrates), ozone, and organic aerosol. Despite its long history of research and the significance of this topic in atmospheric chemistry, a number of important uncertainties remain. These include an incomplete understanding of the rates, mechanisms, and organic aerosol yields for NO3-BVOC reactions, lack of constraints on the role of heterogeneous oxidative processes associated with the NO3 radical, the difficulty of characterizing the spatial distributions of BVOC and NO3 within the poorly mixed nocturnal atmosphere, and the challenge of constructing appropriate boundary layer schemes and non-photochemical mechanisms for use in state-of-the-art chemical transport and chemistry-climate models. This review is the result of a workshop of the same title held at the Georgia Institute of Technology in June 2015. The first half of the review summarizes the current literature on NO3-BVOC chemistry, with a particular focus on recent advances in instrumentation and models, and in organic nitrate and secondary organic aerosol (SOA) formation chemistry. Building on this current understanding, the second half of the review outlines impacts of NO3-BVOC chemistry on air quality and climate, and suggests critical research needs to better constrain this interaction to improve the predictive capabilities of atmospheric models.
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