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A tri-functional metal-organic framework heterogeneous catalyst for efficient conversion of CO2 under mild and co-catalyst free conditions. 2019

Dingxuan Ma, and Yaowen Zhang, and Shaoshao Jiao, and Jixin Li, and Kang Liu, and Zhan Shi
Laboratory of Eco-chemical Engineering, Ministry of Education, College of Chemistry and Molecular Engineering, Qingdao University of Science and Technology, Qingdao 266042, People's Republic of China. madingxuan640@126.com.

Herein, we developed a tri-functional MOF heterogeneous catalyst, MIL-IMAc-Br-, by a post-synthesis modification method for the first time. Due to the synergistic role of three functional sites, including Lewis acid sites, Brønsted acid sites and Br- anion sites, MIL-IMAc-Br- displayed an efficient catalytic performance for the cycloaddition reaction of CO2 and epoxides to form cyclic carbonates under mild and co-catalyst free conditions.

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