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Selective adsorption and separation of C2 hydrocarbons in a "flexible-robust" metal-organic framework based on a guest-dependent gate-opening effect. 2020

Peng-Dan Zhang, and Xue-Qian Wu, and Tao He, and Lin-Hua Xie, and Qiang Chen, and Jian-Rong Li
Beijing Key Laboratory for Green Catalysis and Separation and Department of Chemistry and Chemical Engineering, College of Environmental and Energy Engineering, Beijing University of Technology, Beijing 100124, P. R. China. jrli@bjut.edu.cn.

The selective adsorption/separation of C2 hydrocarbons has been realized in a "flexible-robust" MOF, Zn2(Atz)2Ox. Owing to the distinctive guest-dependent multistep adsorption behaviors and suitable guest-framework interactions, this MOF shows outstanding separation performance for C2H2/C2H4 mixtures in a wide range of temperature confirmed by a column breakthrough experiment.

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