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Rhodium(III)-catalyzed oxidative alkylation of N-aryl-7-azaindoles with cyclopropanols. 2021
Jidan Liu, and
Jinyuan Jiang, and
Zhenke Yang, and
Qiaohai Zeng, and
Jieying Zheng, and
Siying Zhang, and
Liyao Zheng, and
Shang-Shi Zhang, and
Zhao-Qing Liu
School of Chemistry and Chemical Engineering/Institute of Clean Energy and Materials/Guangzhou Key Laboratory for Clean Energy and Materials, Guangzhou University, Guangzhou, 510006, P. R. China. jdliu@gzhu.edu.cn lzqgzu@gzhu.edu.cn.
An efficient Rh(iii)-catalyzed C-H oxidative alkylation of N-aryl-7-azaindoles with cyclopropanols by merging tandem C-H and C-C cleavage was developed. This transformation features mild reaction conditions, high regioselectivity, and excellent functional group compatibility. The resulting β-aryl ketone derivatives can be readily transformed into 7-azaindole-containing π-extended polycyclic heteroarenes.
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